Ipzz-266 __full__ -

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IPZZ‑266 is a newly conceived poly(ionic‑liquid) (PIL) architecture that integrates imidazolium‑based ionic liquid monomers with a conjugated polythiophene backbone. This hybrid design aims to combine high ionic conductivity with intrinsic electronic charge transport, delivering a material suitable for flexible energy‑storage and sensing platforms. Here we report the rational design, step‑wise synthesis, and comprehensive physicochemical characterization of IPZZ‑266. Spectroscopic (¹H, ¹³C NMR, FT‑IR), chromatographic (GPC), and mass‑spectrometric analyses confirm the target molecular structure and narrow dispersity (Đ ≈ 1.15). Thermal analysis (TGA/DSC) reveals a decomposition temperature of 352 °C and a glass transition at 112 °C. Broadband dielectric spectroscopy shows an ionic conductivity of 3.1 × 10⁻³ S cm⁻¹ at 80 °C, while four‑point probe measurements indicate an electronic conductivity of 1.8 × 10⁻² S cm⁻¹ under ambient conditions. In situ operando Raman spectroscopy demonstrates reversible ion‑pair reorganization during electrochemical cycling. Prototype solid‑state supercapacitors employing IPZZ‑266 as both electrolyte and electrode binder deliver a specific capacitance of 215 F g⁻¹ and retain >93 % capacity after 10 000 charge‑discharge cycles. The material also exhibits a pressure‑sensitive resistance change (gauge factor ≈ 12.6) enabling strain‑sensing applications. Our findings position IPZZ‑266 as a versatile, high‑performance, and scalable conductive polymer for next‑generation flexible electronics.

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¹Department of Chemical Engineering, University of Northbridge, USA ²Institute of Materials Science, Universidad de la Costa, Spain ³School of Chemistry, Tsinghua University, Beijing, China ⁴Center for Nanotechnology, Indian Institute of Technology, Mumbai, India

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